WHY is this in Engine Performance + Maintenance instead of Axles + Brakes, or even Stock Suspension?
1. "Adding" grease to an existing bearing is like Russian Roulette. Is the grease you're adding compatible with the grease that's already in there? If not, you're creating potential problems. There's charts on the internet showing the compatibility of various kinds of grease--about a dozen chemical variations, and some mixtures turn evil when combined. The shortest possible story is that some greases are based on clay. They take special, purified clay, mix it with oil, and sell it as "grease". Another popular kind is based on soap. They take special, lithium or calcium soap and mix it with oil, and call it "grease". What do you suppose happens when you apply soap to clay?
For example:
https://www.machinerylubrication.com/Read/1865/grease-compatibility
2. Sure, you can press the hub apart, and maybe even replace the two bearings and races, along with the inner and outer seal. I did, on the '72 Toronado steering knuckles that I used as a disc-brake conversion for my '66 Toro. Problem is, individually the wheel bearings with races are dirt-cheap Maybe seven bucks each. As a matched-pair with spacer, they're expensive--even the "discount" price is forty or fifty bucks. The individual bearings have to be precision-measured, and then supplied with a spacer that goes between them to provide proper end-play. Mix and match bearings, without providing the precision measurements and the specific spacer needed, may or may not get you appropriate bearing clearance once assembled and torqued. You're trusting that the manufacturer is making bearing assemblies that are perfect and uniform to closer than a thousandth of an inch. Good luck.
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3. No way in hell would I replace GM original-equipment bearings with typical aftermarket junk bearings "just because". I'd rather have used-but-usable original equipment parts than bottom-feeder Made In China garbage. If the original bearings feel rough, fine...go to a salvage yard and get used, original bearings that aren't rough. At minimum, buy brand-name bearings and look to see where they're made before shoving the credit card in the reader.